4.6 Article

Large-Area Plasmonic-Crystal-Hot-Electron-Based Photodetectors

Journal

ACS PHOTONICS
Volume 2, Issue 7, Pages 950-957

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.5b00149

Keywords

hot carriers; plasmonic crystal; photodetectors; soft nanoimprint lithography; internal photoemission

Funding

  1. Fundacio Privada Cellex Barcelona
  2. European Commission [PIRG06-GA-2009-256355]
  3. Ministerio de Ciencia e Innovacion [TEC2011-24744]
  4. Nanophotonics for Energy Network of Excellence [N4E GA.248855]
  5. ICFONEST fellowship (COFUND program)

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In view of their exciting optoelectronic light matter interaction properties, plasmonic hot-electron devices have attracted significant attention during the last few years as a novel route for photodetection and light-energy harvesting. Herein we report the use of quasi-3D large-area plasmonic crystals (PC) for hot-electron photodetection, with a tunable response across the visible and near-infrared. The strong interplay between the different PC modes gives access to intense electric fields and hot-carrier generation confined to the metal semiconductor interface, maximizing injection efficiencies with responsivities up to 70 mA/W. Our approach, compatible with large-scale manufacturing, paves the way for the practical implementation of plasmonic hot-electron optoelectronic devices.

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