4.6 Article

Hybrid 2D Material Nanophotonics: A Scalable Platform for Low-Power Nonlinear and Quantum Optics

Journal

ACS PHOTONICS
Volume 2, Issue 8, Pages 1160-1166

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.5b00214

Keywords

nonlinear optics; monolayer material; nanocavity; second order nonlinearity

Funding

  1. National Science Foundation [NSF-EFRI-1433496]
  2. Air Force Office of Scientific Research-Young Investigator Program [FA9550-15-1-0150]
  3. Emerging Frontiers & Multidisciplinary Activities
  4. Directorate For Engineering [1433496] Funding Source: National Science Foundation

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Two-dimensional, atomically thin materials offer unique physical properties, such as a large second-order optical nonlinearity. Integrating these materials into a scalable and silicon-compatible platform could provide a pathway toward realizing low-power nonlinear optics. We have presented a formalism to calculate the effective nonlinear optical coefficient for a cavity integrated 2D material system as well as the cavity enhanced absorptive loss, which can be used to guide future experiments. We have also shown that the few-photon regime of cavity QED is within reach with a cavity quality factor of similar to 10(5)-10(6), provided the loss at the second harmonic mode is minimized. As test applications, we have simulated the performances of (a) an optically bistable device and (b) a nanostructured device exhibiting single-photon blockade.

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