Journal
RSC ADVANCES
Volume 4, Issue 44, Pages 23058-23063Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ra03216k
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Funding
- National Natural Science Foundation of China [51010002, 51272229, 51272231]
- Zhejiang Provincial Natural Science Foundation of China [LR13E020001]
- Qianjiang Talent Project [QJD1302009]
- Welch Foundation [AX1730]
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Hydrocarbons and carbon dioxide are very important raw materials for industrial products and fine chemicals. The microporous metal-organic framework ZJU-25 with high density of open metal sites, has significantly better separation potential than other MOFs, ZIFs or zeolites. It can fractionate a 5-component CH4/C2H2/C2H4/C2H6/CO2 mixture to yield individual pure components as established by the sorption isotherms and simulated breakthrough and pulse chromatographic experiments. Such separations are likely to have a significant industrial impact, resulting in significant energy savings when compared to current technologies that rely on cryogenic distillation.
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