Journal
RSC ADVANCES
Volume 3, Issue 6, Pages 1753-1757Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ra21283h
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Funding
- National Key Basic Research Program of China (973 Program) [2013CB834804]
- Ministry of Science and Technology [2012HFH40090]
- Natural Science Foundation of China (NSFC) [21107117, U1137606]
- Innovative Research Team in University [IRT0979]
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A reduced graphene modified Ta2O5 photocatalyst (Ta2O5-rG) was prepared using a one-step hydrothermal method, and the photocatalytic reduction of an aqueous CO2 solution to CH3OH and H-2 using the NiOx-Ta2O5-rG photocatalyst was performed. Due to graphene's electron transfer and collecting characteristics, reduced graphene was found to be important in achieving high methanol yields for this multi-electron reduction process. The NiOx-Ta2O5-rG photocatalyst also showed good production selectivity for the competing reactions of CH3OH and H-2 generation in aqueous CO2 or CO2/NaHCO3 solution.
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