Journal
RSC ADVANCES
Volume 2, Issue 23, Pages 8645-8652Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ra21487c
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Funding
- National Natural Science Foundation of China [20902046]
- Natural Science Foundation of Jiangsu Province [BK2009384]
- Fundamental Research Funds for the Central Universities [NUST2011ZDJH19]
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The direct N-monomethylation of aromatic primary amines, including arylamines, arylsulfonamides and amino-azoles, using methanol as a methylating agent has been accomplished in the presence of a [Cp*IrCl2](2)/NaOH system. From both synthetic and environmental points of view, the reaction is highly attractive because of low catalyst loading, broad substrate scope and excellent selectivities.
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