Journal
REACTION KINETICS AND CATALYSIS LETTERS
Volume 98, Issue 1, Pages 19-26Publisher
SPRINGER
DOI: 10.1007/s11144-009-0062-9
Keywords
Methane; Syngas; Flow system; Platinum; Oxygen storage material; Single channel
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Funding
- RFBR-CNRS [05-03-34761]
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Partial oxidation of methane (POM) into synthesis gas over a single channel of monolithic catalyst 1.4 wt% Pt/Gd0.3Ce0.35Zr0.35Ox/alpha-Al2O3 was investigated. The effect of the catalyst pretreatment and of the process parameters (temperature, contact time, feed composition) on the catalytic activity and synthesis gas (syngas) selectivity was studied at conditions close to realistic ones with a minimum impact of the mass and heat transfer phenomena. Experimental data are in favor of the direct route of the syngas formation via the methane pyrolysis-selective oxidation sequence.
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