Journal
NANO ENERGY
Volume 15, Issue -, Pages 177-185Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.nanoen.2015.04.030
Keywords
P(VDF-TrFE); Barium titanate (BaTiO3) nanoparticles; Nanocomposite; Piezoelectric nano-generator; Energy storage
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Funding
- Global Frontier Program through the Global Frontier Hybrid Interface Materials (GFHIM) program of the National Research Foundation of Korea (NRF) - Ministry of Science, ICT & Future Planning [2013M3A6B1078872]
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Environmentally friendly and flexible piezoelectric nanogenerators (PENGs) have attracted considerable interest for use in autonomous micro-/nano-systems, wearable electronics, and implantable biomedical devices. Herein, a flexible, lead-free, solution-processable and efficient PENG is demonstrated, based on a highly piezoelectric nanocomposite thin film of barium titanate nanoparticles (BT NPs) embedded into a highly crystalline polyvinylidene fluoride-trifluoroethylene (P(VDF-TrFE)) polymer for charge storage. The nanocomposite PENG (nc-PENG) with high loading of BT NPs up to 40 wt% in the nanocomposite can produce output voltage as high as 9.8 V and output power density of 13.5 mu W/cm2 under cyclic bending, comparable to the output of conventional inorganic polycrystalline lead zirconate titanate PENGs. The high performance of these nc-PENGs is primarily attributed to the very high effective piezoelectricity of the highly crystalline P(VDF-TrFE), strengthened by the BT NPs. The nc-PENG was also demonstrated to harvest biomechanical energy from simple body movements and store the generated electricity during mechanical and biomechanical motions in a rechargeable microbattery. (C) 2015 Elsevier Ltd. All rights reserved.
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