Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 4, Issue 8, Pages 2658-2663Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4cy00250d
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Funding
- National Natural Science Foundation of China [21125314, 21021003, 21373242]
- Chinese Academy of Sciences [KJXC2-YW-H30]
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The Ru/MMT@IL-SO3H catalyst was prepared by immobilizing Ru nanoparticles onto montmorillonite (MMT) with the assistance of an acidic ionic liquid (1-sulfobutyl-3-methylimidazolium hydrosulfate, IL-SO3H). Transmission electron microscopy examination indicated that the loaded Ru species were distributed uniformly on the MMT support with a particle size of about 1.3 nm, which existed mainly in the form of a metallic state as confirmed by X-ray photoelectron spectroscopy analysis. X-Ray diffraction analysis indicated that the interlayer distance of MMT was increased due to the impregnation of IL-SO3H. The activity of Ru/MMT@IL-SO3H for hydrodeoxygenation (HDO) of various phenolic compounds was investigated. It was demonstrated that the as-prepared catalyst served as a bifunctional catalyst and displayed high efficiency for HDO reactions of a series of phenolic compounds to cycloalkanes.
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