Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 3, Issue 1, Pages 99-105Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2cy20561k
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Funding
- CNRS
- European Union for ERC Advanced Grant [NANOSONWINGS 2009-246763]
- Spanish Ministerio de Ciencia e Innovacion [CTQ2010-17476, CSD2007-00006]
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The application of ruthenium nanoparticles (RuNPs) stabilized by the N-heterocyclic carbenes (NHC) N,N'-di(tert-butyl)imidazol-2-ylidene ((IBu)-Bu-t) and 1,3-bis(2,6-diisopropylphenyl)imidazol-2-ylidene IPr as catalysts in the hydrogenation of several substrates is reported under various reaction conditions (solvent, substrate concentration, substrate/metal ratio, temperature). The RuNHC nanoparticles are active catalysts in the hydrogenation of aromatics and show an interesting ligand effect, RuIPr NPs being generally more active than (RuIBu)-Bu-t.
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