Journal
ACS CATALYSIS
Volume 4, Issue 9, Pages 3302-3306Publisher
AMER CHEMICAL SOC
DOI: 10.1021/cs5006597
Keywords
C3N3S3 polymer; graphene; hybrids; metal-free photocatalysis; selective oxidation
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Funding
- NSFC [21003021, 21373051, U1305242]
- Science and Technology project of the Education Office of Fujian Province of P. R. China [JA12017]
- National Basic Research Program of China (973 Program) [2012CB722607]
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Metal-free carbon-based hybrids composed of reduced graphene oxide (rGO) and C3N3S3 polymers with a layered sandwich structure were fabricated by an in situ two-step polymerization strategy and used as visible light photocatalysts for selective aerobic oxygenation of benzylic alcohols to the corresponding aldehydes, at good efficiency and high selectivity. This work shows the great potential and prospective application of the metal-free C3N3S3 polymer in the photocatalyzed synthesis of fine chemicals.
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