Journal
ACS CATALYSIS
Volume 3, Issue 9, Pages 2108-2111Publisher
AMER CHEMICAL SOC
DOI: 10.1021/cs400379h
Keywords
ex situ N-doping; doped carbon nanotubes; aryl-diazonium salt chemistry; electrocatalysts; oxygen reduction reaction (ORR)
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Funding
- Free Cats project [NMP3-SL-2012-280658]
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A straightforward, energy- and atom-saving process to the production of tailored N-doped and catalytically active metal-free carbon nanostructures, has been set up. Our ex situ approach to the N-decoration of the carbon nanotube sidewalls contributes to elucidate the complex structure reactivity relationship of N-doped carbon nanomaterials in oxygen reduction reactions, providing fundamental insights on the nature of the N-active sites as well as on the role of neighboring carbons.
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