Journal
ACS CATALYSIS
Volume 3, Issue 1, Pages 10-13Publisher
AMER CHEMICAL SOC
DOI: 10.1021/cs300682d
Keywords
localized surface plasmon resonance; visible light photocatalysis; Au nanoparticle; selective oxidation; imine synthesis
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Among various metal oxide-supported Au nanoparticles, Au/rutile TiO2 exhibits a particularly high level of visible-light activity for aerobic oxidation of amines to yield the corresponding imines on a synthetic scale with high selectivity (>99%) at 298 K. Experimental results have suggested that the reaction proceeds via the localized surface plasmon resonance-excited electron transfer from the Au nanoparticle to the TiO2.
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