Journal
ACS CATALYSIS
Volume 2, Issue 1, Pages 127-134Publisher
AMER CHEMICAL SOC
DOI: 10.1021/cs200385y
Keywords
hydrodenitrogenation; methylcyclohexylamine; SBA-15; Al-SBA-15; Mo-Ni catalysts
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Funding
- Defence Research and Development Organization (DRDO)
- Department of Science and Technology (DST), New Delhi, India
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Mesoporous Al-SBA-15 with different Si/Al molar ratio (10, 20, 30, and 40) was synthesized hydrothermally, and Mo-Ni catalysts were prepared by incipient wet impregnation method and characterized by different techniques. An impressive catalytic performance was observed on Mo-Ni/Al-SBA-15(10) for Methylcyclohexylamine conversion to hydrocarbons. The observed trend of activity is correlated with the aluminum content, and it is concluded that the variation in Si/Al ratio remarkably affects the hydro-denitrogenation ability of Al-SBA-15 supported Mo-Ni catalysts.
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