Journal
JOURNAL OF MATERIALS CHEMISTRY C
Volume 3, Issue 39, Pages 10188-10194Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5tc01586c
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The investigation of the electrical properties of Co-doped ZnO thin films provides two unexpected results: a decrease of the electrical conductivity and the contemporary occurrence of a reduction of conductivity and of an enhancement of ferromagnetic order. The former result is surprising since Zn atoms are replaced with iso-valent Co atoms. The latter finding questions previously suggested beneficial effects of n-type doping on the ZnO: Co magnetic behavior. While morphological and structural characterization permits us to exclude an influence of the morphology and of the presence of Co metal or Co-oxide phases on present experimental findings, with the aid of first-principles electronic structure calculations, we propose a qualitative picture which can explain in a coherent way both the changes in conductivity and ferromagnetic behavior ensuing from the Co doping and the above-mentioned, beneficial effects of n-type doping.
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