Journal
CHEMICAL SCIENCE
Volume 5, Issue 12, Pages 4554-4560Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4sc01550a
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Funding
- NSFC/China [21322206, 21132005, 91027005, 21302090]
- SMSTC [13JC1402200]
- PCSIRT in University
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The realization of controllable and well-organized self-assembly within multicomponent supramolecular systems (MSSs) is still a great challenge. Herein, we present the construction of multicomponent supramolecular systems with high-level complexity through the combination of orthogonal self-assembly and the self-sorting approach. Driven by the orthogonality of metal-ligand coordination and host-guest interactions in the orthogonal self-assembly as well as directed by multiple molecular codes in the self-sorting process, five types of simple components (up to eighteen precursors) were successfully self-assembled into two novel tris[2]pseudorotaxanes in one pot through a highly selective manner, which were well-characterized by one-dimensional (1-D) and two-dimensional (2-D) multinuclear NMR as well as ESI-TOF-MS.
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