Journal
CHEMICAL SCIENCE
Volume 5, Issue 10, Pages 3803-3807Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4sc01003e
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The first transition metal-free diastereoselective and enantioselective asymmetric allylic alkylation (AAA) has been disclosed leading to the construction of vicinal tertiary/quaternary centers via a kinetic resolution protocol starting from readily available starting materials. This procedure is chemically appealing since no consecutive AAA or stereoselective metal-catalyzed/chiral ligand AAAs are required to construct the two stereocenters.
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