Journal
CHEMICAL SCIENCE
Volume 1, Issue 3, Pages 351-356Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0sc00201a
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Funding
- National Science Foundation/Department of Energy [CHE-0535644]
- U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]
- NSF [DMR 0654118]
- State of Florida
- DOE
- NHMFL [5062]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [0822838, 0848248] Funding Source: National Science Foundation
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Breaking of the carbon-hydrogen bond of benzene and pyridine is observed with (PNP)V(CH(2)tBu)(2) (1), and in the case of benzene, the formation of an intermediate benzyne complex (C) is proposed, and indirect proof of its intermediacy is provided by identification of (PNP)V=O(eta(2)-C(6)H(4)) in combination with DFT calculations.
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