Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 3, Issue 15, Pages 7689-7694Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ta00623f
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Primary Li/FeS2 batteries have been commercialized and rechargeable Li-alloy/FeS2 batteries have been successfully operated at 375-500 degrees C by employing LiCl-based molten electrolytes. However, non-aqueous electrolyte rechargeable Li/FeS2 batteries have not yet been fulfilled due to poor reversibility and rapid capacity fading. The redox mechanism of FeS2 in non-aqueous electrolytes at ambient temperature is poorly understood and is still debated. In this mini-review, we analyse the experimental observations reported previously and propose a suitable mechanism that can explain all of the phenomena observed from the non-aqueous electrolyte Li/FeS2 and Na/FeS2 batteries.
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