Journal
JOURNAL OF ENERGY CHEMISTRY
Volume 24, Issue 2, Pages 207-212Publisher
ELSEVIER
DOI: 10.1016/S2095-4956(15)60302-3
Keywords
carbohydrate biomass; lactic acid; CuO; acetic acid; hydrothermal reactions
Funding
- National Natural Science Foundation of China [21277091]
- State Key Program of National Natural Science Foundation of China [21436007]
- key Basic Research Projects of Science and Technology Commission of Shanghai [14JC1403100]
- Program for Professor of Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher Learning [ZXDF160002]
- SRF for ROCS, SEM [BG1600002]
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An improved two-step process for converting carbohydrate biomass to acetic acid under hydrothermal conditions is proposed. The first step consists of the production of lactic acid from carbohydrate biomass, and the second step consists of conversion of the lactic acid obtained in the first step to acetic acid using CuO as an oxidant. The results indicated that CuO as an oxidant in the second step can significantly improve the production of high-purity acetic acid from lactic acid, and the maximum yield of acetic acid was 61%, with a purity of 90%. The yield of acetic acid obtained using the improved two-step hydrothermal process from carbohydrate biomass, such as glucose, cellulose and starch, was greater than that obtained using traditional two-step process with H2O2 or O-2. In addition, a proposed pathway for the production of acetic acid from lactic acid in the second step with CuO was also discussed. The present study provides a useful two-step process for the production of acetic acid from carbohydrate biomass.
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