4.4 Review

Recent Advances in Voltammetry

Journal

CHEMISTRYOPEN
Volume 4, Issue 3, Pages 224-260

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/open.201500042

Keywords

cyclic voltammetry; electrochemistry; electron transfer; kinetics; mass transport; nanoparticle electrochemistry; stripping voltammetry

Funding

  1. European Research Council (ERC) under the European Unions Seventh Framework Programme (FP) [320403]
  2. Ministerio de Economia y Competitividad, Spain [CTQ2012-36700]
  3. European Regional Development Fund
  4. Fundacion Seneca de la Region de Murcia [18968/JLI/13]
  5. European Union Seventh Framework Programme-Marie Curie COFUND (FP7) under University of Murcia Incoming Mobility Programme Action (U-IMPACT)

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Recent progress in the theory and practice of voltammetry is surveyed and evaluated. The transformation over the last decade of the level of modelling and simulation of experiments has realised major advances such that electrochemical techniques can be fully developed and applied to real chemical problems of distinct complexity. This review focuses on the topic areas of: multistep electrochemical processes, voltammetry in ionic liquids, the development and interpretation of theories of electron transfer (Butler-Volmer and Marcus-Hush), advances in voltammetric pulse techniques, stochastic random walk models of diffusion, the influence of migration under conditions of low support, voltammetry at rough and porous electrodes, and nanoparticle electrochemistry. The review of the latter field encompasses both the study of nanoparticle-modified electrodes, including stripping voltammetry and the new technique of 'nano-impacts'.

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