Journal
TOPICS IN CATALYSIS
Volume 53, Issue 15-18, Pages 1132-1137Publisher
SPRINGER/PLENUM PUBLISHERS
DOI: 10.1007/s11244-010-9546-0
Keywords
Iridium; Palladium; Bimetallic catalysts; Benzonitrile; Hydrogenation
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Funding
- National Action Council for Minorities in Engineering (NACME), Inc.
- NSF
- SEAGEP
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The kinetics of liquid-phase hydrogenation of benzonitrile have been examined alumina supported Ir, Pd and Ir-Pd catalysts. Benzonitrile disappearance TOF is 10-fold higher for Pd catalyst than it is for Ir catalyst. Benzylamine is produced preferentially over Pd, whereas dibenzylamine is produced principally over Ir. Non-monotonic activity and selectivity relationships with bimetallic composition are obtained.
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