Journal
THEORETICAL AND EXPERIMENTAL CHEMISTRY
Volume 46, Issue 1, Pages 32-38Publisher
SPRINGER
DOI: 10.1007/s11237-010-9117-2
Keywords
acetylene; hydrochlorination; heterogeneous catalysis; active sites; palladium(II) complexes; mechanical activation
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Funding
- National Academy of Sciences of Ukraine [0101U008137]
- Ukraine Ministry of Education and Science [0103I003614]
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A heterogeneous catalyst for the hydrochlorination of acetylene using gaseous HCl was obtained by prior mechanical activation of K2PdCl4 powder in an atmosphere of acetylene or propylene. Active sites are formed during the mechanical treatment in the surface layers of the catalyst, which are Pd(II) complexes with a coordination vacancy.
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