Journal
TETRAHEDRON
Volume 69, Issue 23, Pages 4708-4724Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2013.03.073
Keywords
alpha-Aminophosphonates; Carbon nanotubes; Heterogeneous catalyst; Iron-doped; Organophosphorus; beta-Phosphonomalonates; Solvent free
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Funding
- Shiraz University Research Council
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Iron-doped single walled carbon nanotubes (Fe/SWCNTs) is an efficient, eco-friendly, and reusable heterogeneous catalyst for the synthesis of diversely decorated alpha-aminophosphonates via multicomponent reaction of amines, carbonyl compounds, and phosphorus compounds under solvent-free conditions. This methodology illustrates a very simple procedure, with wide applicability, extending the scope to aliphatic and aromatic amines and carbonyl compounds. It also enabled the development of one-pot synthesis of beta-phosphonomalonates during the reaction of carbonyl compounds, malononitrile and phosphorus compounds. Excellent results were obtained in each case affording the corresponding organophosphorus adducts in good yields. (C) 2013 Elsevier Ltd. All rights reserved.
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