Journal
TETRAHEDRON
Volume 68, Issue 46, Pages 9376-9383Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2012.09.034
Keywords
Alkaloid; Benzyne; Cyclization; One-pot reaction; Pyrroloquinoline
Categories
Funding
- Cabinet Office, Government of Japan [LS008]
- Ministry of Education, Culture, Sports, Science, and Technology, Japan
- KAKENHI [19890014, 21790006, 23790004]
- Tohoku University
- Nagase Science and Technology Foundation
- Suntory Institute for Bioorganic Research
- Astellas Foundation for Research on Metabolic Disorders
- Banyu Life Science Foundation International
- Grants-in-Aid for Scientific Research [19890014, 23790004, 21790006] Funding Source: KAKEN
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Total synthesis of pyrroloquinoline alkaloids, such as makaluvamine AID, damirone B, batzelline C, makaluvone, and isobatzelline C, was achieved featuring a one-pot benzyne-mediated cyclization-functionalization reaction. The synthetic utility was demonstrated by the construction of the common pyrrolo[4,3,2-de]quinoline skeleton. (C) 2012 Elsevier Ltd. All rights reserved.
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