Journal
TETRAHEDRON
Volume 67, Issue 5, Pages 877-880Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2010.12.015
Keywords
Biosynthesis; Ladder-frame polyether; C-13-Labeling; Carbon deletion
Categories
Funding
- Global COE Program for Chemistry Innovation
- University of Tokyo
- KAKENHI
- Grants-in-Aid for Scientific Research [22404006] Funding Source: KAKEN
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Biosynthesis of a marine ladder-frame polyether yessotoxin (YTX) produced by the dinofalgellate Protoceratium reticulatum was investigated. The C-13-labeling experiments indicated that the carbons in YTX were derived from acetates, a methyl of methionine and glycolate, and six-membered ring tetrads (rings A-D and H-K) were constructed from repetition of C3 units (m-m-c), which consisted of a methyl of acetate and acetate. (C) 2010 Elsevier Ltd. All rights reserved.
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