4.3 Article

FACILE ACCESS TO 3-ALKYL-SUBSTITUTED 3-HYDROPEROXY-2,4-PYRROLIDINEDIONES USING MANGANESE(III)-CATALYZED AEROBIC OXIDATION

Journal

SYNTHETIC COMMUNICATIONS
Volume 42, Issue 4, Pages 608-619

Publisher

TAYLOR & FRANCIS INC
DOI: 10.1080/00397911.2010.528129

Keywords

Aerobic oxidation; catalytic oxidation; hydroperoxidation; hydroperoxypyrrolidinediones; manganese(III) acetate; 2,4-pyrrolidinediones

Funding

  1. Japan Society for the Promotion of Science [19550046]
  2. Grants-in-Aid for Scientific Research [22550041] Funding Source: KAKEN

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3-Alkyl-substituted 2,4-pyrrolidinediones were directly oxidized under very mild manganese(III)-catalyzed aerobic oxidation conditions to give the corresponding 3-hydroperoxy-2,4-pyrrolidinediones in quantitative yields. The scope and limitations for the synthesis of the hydroperoxyprrolidinediones are described.

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