Journal
SYNTHESIS-STUTTGART
Volume 46, Issue 14, Pages 1853-1858Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0033-1339109
Keywords
aryl methyl ketones; DMF; copper; oxygen; alpha-ketoamides
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Funding
- National Science Foundation of China [21202049]
- Recruitment Program of Global Experts (1000 Talents Plan), Fujian Hundred Talents Program, and Research Funds of Huaqiao University
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A copper-catalyzed aerobic oxidative coupling of aryl methyl ketones with N,N-dimethylformamide was developed, which afforded alpha-ketoamides by a sequence of dioxygen activation, C-H bond functionalization, and amide formation with N, N-dimethylformamide as the nitrogen source. Molecular oxygen was found to play a crucial role in this transformation.
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