Journal
SYNTHESIS-STUTTGART
Volume -, Issue 21, Pages 3423-3428Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0028-1083177
Keywords
Pd/C/K-10 montmorillonite; solid acid; microwave irradiation; bifunctional catalysis; green chemistry; pyridines
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Funding
- University of Massachusetts Boston
- ACS PRF
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A one-pot synthesis of substituted pyridines via a domino cyclization-oxidative aromatization (dehydrogenation) approach is described. The process is based on the use of a new bifunctional noble metal-solid acid catalyst, Pd/C/K-10 montmorillonite and microwave irradiation. The cyclization readily takes place on the strong solid acid while palladium dehydrogenates the dihydropyridine intermediates to the desired products.
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