Journal
SYNLETT
Volume 25, Issue 5, Pages 713-717Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0033-1340669
Keywords
acetals; desymmetrization; Michael addition; stereoselective synthesis; cascade catalysis
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Funding
- NIGMS [GM72586]
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The desymmetrization of p-quinols using a Bronsted acid catalyzed acetalization/Michael cascade was achieved in high yields and diastereoselectivities for aldehydes and imines. Use of a chiral Bronsted acid allowed for the synthesis of 1,3-dioxolane and 1,3-oxazolidine products in modest enantioselectivity.
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