Journal
SYNLETT
Volume 25, Issue 6, Pages 783-794Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0033-1340618
Keywords
asymmetric catalysis; amines; acylation; kinetic resolution; desymmetrization
Categories
Funding
- National Science Foundation [CHE-1300382]
- Alexander von Humboldt Foundation
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1300382] Funding Source: National Science Foundation
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This account details the development of a dual-catalysis approach and its application to the kinetic resolution of amines and other enantioselective acyl-transfer reactions. Anion recognition is an essential design element of these processes, which are enabled by the combined action of an achiral 4-(N,N-dimethylamino)pyridine (DMAP) derivative and a chiral anion receptor catalyst.
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