Journal
CHEMPLUSCHEM
Volume 81, Issue 2, Pages 187-193Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cplu.201500382
Keywords
coordination complexes; electrochemical deposition; europium; luminescence; thin films
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Funding
- Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan [2401, 24102012]
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Luminescent thin films composed of thermostable lanthanide coordination polymers on glass electrodes were prepared using a novel combination of micelle reactions and electrochemical deposition techniques. The micelle-encapsulated luminescent polymers were obtained by the polymerization of [Eu(hfa)(3)] (hfa=hexafluoroacetylacetonate) with bridging phosphine oxide ligands in micelles using a redox-active ferrocenyl-containing surfactant in water. Films were electrochemically deposited on indium tin oxide coated glass electrodes by potentiostatic polarization of micelle-encapsulated Eu-III coordination polymers. The luminescence properties of the electrochemically deposited films were characterized by measuring their emission spectra, emission lifetimes and emission quantum yields.
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