Journal
ACS MACRO LETTERS
Volume 4, Issue 10, Pages 1163-1168Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsmacrolett.5b00608
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Funding
- European Regional Development Fund
- Republic of Cyprus through Cyprus Research Promotion Foundation [IPE/NEKYP/0311/27, 0308/02]
- European Research Council (ERC) [336839]
- neutron beam time at Institut Laue-Langevin (ILL) Grenoble, France
- Julich Center for Neutron Science (JCNS), Garching Germany
- National Institute of Standards and Technology (NIST), Gaithersburg, Maryland
- European Research Council (ERC) [336839] Funding Source: European Research Council (ERC)
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Amphiphilic polymer conetworks are cross-linked polymers that swell both in water and in organic solvents and can phase separate on the nanoscale in the bulk or in selective solvents. To date, however, this phase separation has only been reported with short-range order, characterized by disordered morphologies. We now report the first example of amphipliilic polymer conetworks, based on end-linked core-first star block copolymers, that form a lamellar phase with long-range order. These mesoscopically ordered systems can be produced in a simple fashion and exhibit significantly improved mechanical properties.
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