4.6 Article

Partial universality: pinch-off dynamics in fluids with smectic liquid crystalline order

Journal

SOFT MATTER
Volume 6, Issue 5, Pages 892-895

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/b923069f

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Funding

  1. Procter and Gamble Company [NSF-DMR 0606040, NSF-CMMI 0726773]

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Droplet pinch-off of fluids with liquid crystalline order is a common yet poorly understood process. We report on measurements of pinch-off dynamics for a lyotropic surfactant/water solution in the lamellar phase and a thermotropic liquid crystal in the smectic phase. We find pinch-off is universal and well described by a similarity solution for a strain thinning power-law fluid. This finding is consistent with bulk rheology measurements which show these materials shear thin with the appropriate power-law dependence. Remarkably, we find depending on material processing, this universal pinch-off cuts off at different length scales. Collectively, these phenomena lead to an exceptional form of singularity where pinch-off is both universal and dependent on initial conditions.

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