Journal
RSC ADVANCES
Volume 5, Issue 34, Pages 26675-26679Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ra02816g
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Funding
- Main Direction Program of Knowledge Innovation of Chinese Academy of Sciences [KGCX2-YW-399+11]
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Melem and its derivatives were synthesized from melamine by a two-step heat treatment method between 400 and 650 degrees C in air. It was demonstrated that such polymeric C-N semiconductors possess a photoelectrochemical (PEC) conversion effect with both photocathodic and photoanodic characteristics, which was proposed to be caused by the formation of tri-s-triazine ring. The dimelem synthesized at 450 degrees C exhibited the highest PEC conversion activity. The possible reasons were discussed. The unique bidirectional photocurrent generation makes melem and its derivatives attractive photoelectrochemical materials.
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