Journal
SCIENCE
Volume 345, Issue 6196, Pages 542-546Publisher
AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/science.1254050
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Funding
- NSF [ECCS-1202231]
- Air Force Office of Scientific Research [FA9550-12-1-0074]
- UCLA
- Directorate For Engineering [1202231] Funding Source: National Science Foundation
- Div Of Electrical, Commun & Cyber Sys [1202231] Funding Source: National Science Foundation
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Advancing perovskite solar cell technologies toward their theoretical power conversion efficiency (PCE) requires delicate control over the carrier dynamics throughout the entire device. By controlling the formation of the perovskite layer and careful choices of other materials, we suppressed carrier recombination in the absorber, facilitated carrier injection into the carrier transport layers, and maintained good carrier extraction at the electrodes. When measured via reverse bias scan, cell PCE is typically boosted to 16.6% on average, with the highest efficiency of similar to 19.3% in a planar geometry without antireflective coating. The fabrication of our perovskite solar cells was conducted in air and from solution at low temperatures, which should simplify manufacturing of large-area perovskite devices that are inexpensive and perform at high levels.
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