Journal
RSC ADVANCES
Volume 5, Issue 64, Pages 52066-52071Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ra07072d
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Funding
- State 863 project [2012AA062803]
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Porous Co3O4-MOF and Ru/Co3O4-MOF were prepared through a metal-organic frameworks (MOFs)-templated method, and the bulk materials resulted from precipitation method were prepared for comparison. All catalysts were tested for the catalytic oxidation of toluene in the temperature range of 150-300 degrees C, and Ru/Co3O4-MOF showed apparently higher catalytic activity and CO2 selectivity than other materials. The influence of water vapour on the catalytic oxidation of toluene was studied at 235 degrees C and 245 degrees C, and it could be found that the inhibition effect weakened with the increase of temperature. Additionally, the test of 12 h on-stream reaction was conducted to explore the stability of Ru/Co3O4-MOF.
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