Journal
RSC ADVANCES
Volume 5, Issue 82, Pages 66994-67000Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ra12377a
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Funding
- National Basic Research Program China [2013CB932902]
- National Natural Science Foundation of China [51103023, 21173042]
- Scientific Research Foundation of Graduate School of Southeast University
- Fundamental Research Funds for the Central Universities
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A novel bipolar material featuring triphenylamine and benzimidazole groups has been designed and synthesized. The unique star-shaped configuration enables the materials with high thermal stability and a film-forming property. Both DFT simulation and experimental results demonstrated that the enhanced electron affinity and transporting ability endows the solution-processed devices based on TPA-2PBI with more balanced charge flux and higher exciton recombination efficiency. As a result, the non-doped deep blue electrofluorescent device using TPA-2PBI as the emitter shows the maximum luminance efficiency of 1.53 cd A(-1) and the green electrophosphorescent device using TPA-2PBI as the host material shows the maximum luminance efficiency of 38.0 cd A(-1). Furthermore, the TPA-2PBI based devices exhibit higher performance compared with the corresponding devices based on 2TPA-PBI.
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