4.5 Article

An innovative Yb-based ultrafast deep ultraviolet source for time-resolved photoemission experiments

Journal

REVIEW OF SCIENTIFIC INSTRUMENTS
Volume 85, Issue 12, Pages -

Publisher

AMER INST PHYSICS
DOI: 10.1063/1.4903347

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Funding

  1. Fondazione Cariplo
  2. EC under Graphene Flagship [CNECT-ICT-604391]
  3. MIUR FIRB Grant [RBFR12SW0J]

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Time- and angle-resolved photoemission spectroscopy is a powerful technique to study ultrafast electronic dynamics in solids. Here, an innovative optical setup based on a 100-kHz Yb laser source is presented. Exploiting non-collinear optical parametric amplification and sum-frequency generation, ultrashort pump (h nu = 1.82 eV) and ultraviolet probe (h nu = 6.05 eV) pulses are generated. Overall temporal and instrumental energy resolutions of, respectively, 85 fs and 50 meV are obtained. Time- and angle-resolved measurements on BiTeI semiconductor are presented to show the capabilities of the setup. (C) 2014 AIP Publishing LLC.

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