100-femtosecond MeV electron source for ultrafast electron diffraction

A near-relativistic 100-fs MeV electron beam is developed by using a photocathode rf gun for revealing the hidden ultrafast dynamics of intricate molecular and atomic processes in materials through experimentation of ultrafast time-resolved electron diffraction (LIED). The transverse and longitudinal dynamics of femtosecond electron beam in the rf gun were studied theoretically by particle simulation. The growths of the emittance, bunch length and energy spread due to the rf and space charge effects were investigated by changing the laser parameters, field gradient and electron charge. The theoretical studies indicate that a 100-fs MeV electron beam with the transverse emittance of 0.1 mm mrad and the relative energy spread of 10(-3)-10(-4) at bunch charge of 0.1-2 pC (10(6)-10(7) electrons per pulse) is achievable for LIED, in which the intensity is three orders of magnitude higher than that produced by the conventional dc or pulsed guns. (C) 2009 Elsevier Ltd. All rights reserved.