Journal
PURE AND APPLIED CHEMISTRY
Volume 80, Issue 4, Pages 727-742Publisher
WALTER DE GRUYTER GMBH
DOI: 10.1351/pac200880040727
Keywords
total synthesis; natural products; marine neurotoxins; antibiotics; antitumor agents
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Total synthesis campaigns toward complex heterocyclic natural products are a prime source of inspiration for the design and execution of complex cascade sequences, powerful reactions, and efficient synthetic strategies. We highlight selected examples of such innovations in the course of our total syntheses of diazonamide A, azaspiracid-1, thiostrepton, 2,2'-epi-cytoskyrin A and rugulosin, abyssomicin C, platensimycin, and uncialamycin.
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