Journal
ACS CATALYSIS
Volume 5, Issue 8, Pages 4556-4567Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.5b00757
Keywords
porous organic polymers; covalent organic frameworks; heterogeneous catalysis; metal-free polymerization; adjustable wettability
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Funding
- National Natural Science Foundation of China [21422306, 21333009, 21273197]
- National High-Tech Research and Development Program of China [2013AA065301]
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Porous organic polymers (POPs), which feature high surface areas and designable pore walls, have attracted much attention recently as a result of combining the advantages of both heterogeneous and homogeneous catalysts. Because of the diversity of chemical reactions, one could design polymer frameworks with unique functionalities used as active sites and ligands in catalysis. In the view of green chemistry, this perspective is focused mainly on rational preparation of the porous organic polymers under metal-free conditions and their applications in heterogeneous catalysis. It is observed that many POP-based heterogeneous catalysts demonstrate superior catalytic properties, even better than the homogeneous counterparts. The strategies for designing highly efficient heterogeneous catalysts are briefly assessed.
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