4.8 Article

Single-shot stand-off chemical identification of powders using random Raman lasing

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.1412535111

Keywords

remote sensing; Raman spectroscopy; stimulated Raman scattering; stand-off detection

Funding

  1. National Science Foundation (NSF) [ECCS-1250360, DBI-1250361, CBET-1250363, PHY-1241032, ECC-0540832]
  2. Robert A. Welch Foundation [A-1261]
  3. Directorate For Engineering
  4. Div Of Chem, Bioeng, Env, & Transp Sys [1250363] Funding Source: National Science Foundation
  5. Directorate For Engineering
  6. Div Of Electrical, Commun & Cyber Sys [1250360] Funding Source: National Science Foundation
  7. Division Of Physics
  8. Direct For Mathematical & Physical Scien [1241032] Funding Source: National Science Foundation
  9. Div Of Biological Infrastructure
  10. Direct For Biological Sciences [1250361] Funding Source: National Science Foundation

Ask authors/readers for more resources

The task of identifying explosives, hazardous chemicals, and biological materials from a safe distance is the subject we consider. Much of the prior work on stand-off spectroscopy using light has been devoted to generating a backward-propagating beam of light that can be used drive further spectroscopic processes. The discovery of random lasing and, more recently, random Raman lasing provide a mechanism for remotely generating copious amounts of chemically specific Raman scattered light. The bright nature of random Raman lasing renders directionality unnecessary, allowing for the detection and identification of chemicals from large distances in real time. In this article, the single-shot remote identification of chemicals at kilometer-scale distances is experimentally demonstrated using random Raman lasing.

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