4.8 Article

Many-body interactions in quasi-freestanding graphene

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.1100242108

Keywords

band structure; dielectric screening; fine structure constant; density functional theory; self-energy

Funding

  1. Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy [DE-AC02-05CH11231]
  2. Office of Naval Research Multidisciplinary University Initiative [N00014-09-1-1066]
  3. Materials Research Science and Engineering Centers under National Science Foundation [DMR-0820382]
  4. National Science Foundation [DMR10-1006184]
  5. Direct For Mathematical & Physical Scien
  6. Division Of Materials Research [1006184] Funding Source: National Science Foundation

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The Landau-Fermi liquid picture for quasiparticles assumes that charge carriers are dressed by many-body interactions, forming one of the fundamental theories of solids. Whether this picture still holds for a semimetal such as graphene at the neutrality point, i.e., when the chemical potential coincides with the Dirac point energy, is one of the long-standing puzzles in this field. Here we present such a study in quasi-freestanding graphene by using high-resolution angle-resolved photoemission spectroscopy. We see the electron-electron and electron-phonon interactions go through substantial changes when the semimetallic regime is approached, including renormalizations due to strong electron-electron interactions with similarities to marginal Fermi liquid behavior. These findings set a new benchmark in our understanding of many-body physics in graphene and a variety of novel materials with Dirac fermions.

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