4.8 Article

Visualizing the formation of the Kondo lattice and the hidden order in URu2Si2

Publisher

NATL ACAD SCIENCES
DOI: 10.1073/pnas.1005892107

Keywords

heavy fermion; scanning tunneling spectroscopy

Funding

  1. Department of Energy Basic Energy Sciences
  2. National Science Foundation
  3. W. M. Keck Foundation
  4. Division Of Materials Research
  5. Direct For Mathematical & Physical Scien [819860] Funding Source: National Science Foundation

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Heavy electronic states originating from the f atomic orbitals underlie a rich variety of quantum phases of matter. We use atomic scale imaging and spectroscopy with the scanning tunneling microscope to examine the novel electronic states that emerge from the uranium f states in URu2Si2. We find that, as the temperature is lowered, partial screening of the f electrons' spins gives rise to a spatially modulated Kondo-Fano resonance that is maximal between the surface U atoms. At T = 17.5 K, URu2Si2 is known to undergo a second-order phase transition from the Kondo lattice state into a phase with a hidden order parameter. From tunneling spectroscopy, we identify a spatially modulated, bias-asymmetric energy gap with a mean-field temperature dependence that develops in the hidden order state. Spectroscopic imaging further reveals a spatial correlation between the hidden order gap and the Kondo resonance, suggesting that the two phenomena involve the same electronic states.

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