Journal
PHYSICAL REVIEW LETTERS
Volume 112, Issue 2, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.112.027202
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Funding
- U.S. Department of Energy, office of Basic Energy Sciences, Division of Material Sciences and Engineering [DE-FG02-08ER46544]
- National Science Foundation [DMR-0944772]
- U.S. Department of Energy, office of Basic Energy Sciences, Scientific User Facilities Division
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Inelastic neutron scattering at low temperatures T <= 30 K from a powder of LiZn2Mo3O8 demonstrates this triangular-lattice antiferromagnet hosts collective magnetic excitations from spin-1/2 Mo3O13 molecules. Apparently gapless (Delta < 0.2 meV) and extending at least up to 2.5 meV, the low-energy magnetic scattering cross section is surprisingly broad in momentum space and involves one-third of the spins present above 100 K. The data are compatible with the presence of valence bonds involving nearest-neighbor and next-nearest-neighbor spins forming a disordered or dynamic state.
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