Journal
PHYSICAL REVIEW LETTERS
Volume 111, Issue 12, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.111.123002
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Funding
- Engineering and Physical Sciences Research Council (EPSRC, UK) [EP/H003657/1]
- EPSRC through the Programme Grant on Attosecond Dynamics [EP/I032517]
- CORINF
- Marie Curie ITN of the European Union [264951]
- ERC Advanced Grant ASTEX [290467]
- EPSRC [EP/H003657/1, EP/I032517/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/I032517/1, EP/H003657/1] Funding Source: researchfish
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We show how high-order harmonic generation spectroscopy can be used to follow correlation-driven electron hole dynamics with attosecond time resolution. The technique is applicable both to normal Auger transitions and to electron hole migration processes that do not lead to secondary electron emission. We theoretically simulate the proposed spectroscopy for M4,5NN Auger decay in Kr and for correlation-driven inner-valence hole dynamics in trans-butadiene and propanal.
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