4.8 Article

Measurement of Filling-Factor-Dependent Magnetophonon Resonances in Graphene Using Raman Spectroscopy

Journal

PHYSICAL REVIEW LETTERS
Volume 110, Issue 22, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.110.227402

Keywords

-

Funding

  1. NHMFL [UCGP-5068]
  2. DOE/BES [DE-FG02-07ER46451, DE-FG02-06ER46308]
  3. Robert A. Welch Foundation [C-1509]
  4. EPSRC [GR/S97613/01, EP/E500935/1, EP/K01711X/1, EP/K017144/1, EP/G042357/1]
  5. ERC
  6. EU
  7. Leverhulme Trust
  8. NSF ECCS [0925988]
  9. ERC AdG Graphene and Beyond''
  10. NSF [DMR-0654118]
  11. State of Florida
  12. DOE
  13. Royal Society
  14. Direct For Mathematical & Physical Scien
  15. Division Of Materials Research [1006663] Funding Source: National Science Foundation
  16. Div Of Electrical, Commun & Cyber Sys
  17. Directorate For Engineering [0925988] Funding Source: National Science Foundation
  18. Engineering and Physical Sciences Research Council [EP/G042357/1, EP/G035954/1, GR/S97613/01, EP/K01711X/1, EP/K017144/1, EP/E500935/1] Funding Source: researchfish
  19. EPSRC [EP/G035954/1, EP/K01711X/1, EP/K017144/1, EP/G042357/1, EP/E500935/1] Funding Source: UKRI

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We perform polarization-resolved Raman spectroscopy on graphene in magnetic fields up to 45 T. This reveals a filling-factor-dependent, multicomponent anticrossing structure of the Raman G peak, resulting from magnetophonon resonances between magnetoexcitons and E-2g phonons. This is explained with a model of Raman scattering taking into account the effects of spatially inhomogeneous carrier densities and strain. Random fluctuations of strain-induced pseudomagnetic fields lead to increased scattering intensity inside the anticrossing gap, consistent with the experiments.

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