Journal
PHYSICAL REVIEW LETTERS
Volume 109, Issue 13, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.109.133001
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- Chemical Sciences, Geo-Sciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy
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We describe a pump-probe scheme with which the spatial asymmetry of dissociating molecular fragments-as controlled by the carrier-envelope phase of an intense few-cycle laser pulse-can be enhanced by an order of magnitude or more. We illustrate the scheme using extensive, full-dimensional calculations for dissociation of H-2(+) and include the averaging necessary for comparison with experiment.
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