Journal
PHYSICAL REVIEW LETTERS
Volume 105, Issue 11, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.105.113002
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Funding
- National Science Foundation [CHE-0647913]
- Research Corporation Cottrell Scholar
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Lack of memory (locality in time) is a major limitation of almost all present time-dependent density-functional approximations. By using semiclassical dynamics to compute correlation effects in the time propagation of the density matrix, we incorporate memory, including initial-state dependence, as well as changing occupation numbers, and predict more observables in strong-field applications.
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