Evidence for Electroactive Excitation of the Spin Cycloid in TbMnO3

Terahertz electromagnetic excitations in the multiferroic TbMnO3 single crystals are investigated across the magnetic field induced rotation of the magnetic spin cycloid. In addition to the electromagnon along the a axis, the detailed polarization analysis of the experimental spectra suggests the existence of an electroactive excitation for ac electric fields of the electromagnetic wave along the crystallographic c axis. This excitation is possibly the electroactive eigenmode of the spin-cycloid in TbMnO3, which has been predicted within the inverse Dzyaloshinskii-Moriya mechanism of magnetoelectric coupling.